Ni3S2/Ni-P bilayer coated on polyimide as a Pt- and TCO-free flexible counter electrode for dye-sensitized solar cells.
Identifieur interne : 000104 ( Main/Exploration ); précédent : 000103; suivant : 000105Ni3S2/Ni-P bilayer coated on polyimide as a Pt- and TCO-free flexible counter electrode for dye-sensitized solar cells.
Auteurs : RBID : pubmed:24446929Abstract
In this study, we reported an efficient, flexible, and low-cost (Pt-free and transparent conducting oxide (TCO)-free) counter electrode (CE) made of a polyimide (PI) substrate coated with a Ni3S2/Ni-P bilayer for dye-sensitized solar cells (DSCs). The bilayer Ni3S2/Ni-P hybrid film was deposited on a PI plastic substrate via a series of wet chemical/electrochemical processes. The bottom Ni-P layer was deposited on a PI to replace conventional TCO as a conductive layer, and the top Ni3S2 layer was employed as the electrocatalyst for I3(-) reduction. On the basis of the extensive electrochemical measurments, the as-prepared Ni3S2/Ni-P coated PI flexible CE demonstrated a Pt-like electrocatalytic for I3(-) reduction. As a result, the DSC assembled with the Ni3S2/Ni-P coated PI flexible CE exhibited an impressive photovoltaic conversion efficiency of 6.28% accompanied by a fill factor of 0.63 under 1 sun illumination (100 mW cm(-2), AM 1.5), which is comparative to that of the DSC based on the Pt coated indium tin oxide/polyethylene naphthalate (ITO/PEN) CE.
DOI: 10.1021/am405384c
PubMed: 24446929
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Ni3S2/Ni-P bilayer coated on polyimide as a Pt- and TCO-free flexible counter electrode for dye-sensitized solar cells.</title><author><name sortKey="Lin, Jeng Yu" uniqKey="Lin J">Jeng-Yu Lin</name><affiliation wicri:level="1"><nlm:affiliation>Department of Chemical Engineering, Tatung University , No. 40, Sec. 3, ChungShan North Road, Taipei City 104, Taiwan.</nlm:affiliation><country xml:lang="fr">République de Chine (Taïwan)</country><wicri:regionArea>Department of Chemical Engineering, Tatung University , No. 40, Sec. 3, ChungShan North Road, Taipei City 104</wicri:regionArea></affiliation></author><author><name sortKey="Wang, Wei Yan" uniqKey="Wang W">Wei-Yan Wang</name></author><author><name sortKey="Lin, Yi Ting" uniqKey="Lin Y">Yi-Ting Lin</name></author><author><name sortKey="Chou, Shu Wei" uniqKey="Chou S">Shu-Wei Chou</name></author></titleStmt><publicationStmt><date when="2014">2014</date><idno type="doi">10.1021/am405384c</idno><idno type="RBID">pubmed:24446929</idno><idno type="pmid">24446929</idno><idno type="wicri:Area/Main/Corpus">000203</idno><idno type="wicri:Area/Main/Curation">000203</idno><idno type="wicri:Area/Main/Exploration">000104</idno></publicationStmt></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">In this study, we reported an efficient, flexible, and low-cost (Pt-free and transparent conducting oxide (TCO)-free) counter electrode (CE) made of a polyimide (PI) substrate coated with a Ni3S2/Ni-P bilayer for dye-sensitized solar cells (DSCs). The bilayer Ni3S2/Ni-P hybrid film was deposited on a PI plastic substrate via a series of wet chemical/electrochemical processes. The bottom Ni-P layer was deposited on a PI to replace conventional TCO as a conductive layer, and the top Ni3S2 layer was employed as the electrocatalyst for I3(-) reduction. On the basis of the extensive electrochemical measurments, the as-prepared Ni3S2/Ni-P coated PI flexible CE demonstrated a Pt-like electrocatalytic for I3(-) reduction. As a result, the DSC assembled with the Ni3S2/Ni-P coated PI flexible CE exhibited an impressive photovoltaic conversion efficiency of 6.28% accompanied by a fill factor of 0.63 under 1 sun illumination (100 mW cm(-2), AM 1.5), which is comparative to that of the DSC based on the Pt coated indium tin oxide/polyethylene naphthalate (ITO/PEN) CE.</div></front></TEI><pubmed><MedlineCitation Owner="NLM" Status="In-Process"><PMID Version="1">24446929</PMID><DateCreated><Year>2014</Year><Month>03</Month><Day>12</Day></DateCreated><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1944-8252</ISSN><JournalIssue CitedMedium="Internet"><Volume>6</Volume><Issue>5</Issue><PubDate><Year>2014</Year><Month>Mar</Month><Day>12</Day></PubDate></JournalIssue><Title>ACS applied materials & interfaces</Title><ISOAbbreviation>ACS Appl Mater Interfaces</ISOAbbreviation></Journal><ArticleTitle>Ni3S2/Ni-P bilayer coated on polyimide as a Pt- and TCO-free flexible counter electrode for dye-sensitized solar cells.</ArticleTitle><Pagination><MedlinePgn>3357-64</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/am405384c</ELocationID><Abstract><AbstractText>In this study, we reported an efficient, flexible, and low-cost (Pt-free and transparent conducting oxide (TCO)-free) counter electrode (CE) made of a polyimide (PI) substrate coated with a Ni3S2/Ni-P bilayer for dye-sensitized solar cells (DSCs). The bilayer Ni3S2/Ni-P hybrid film was deposited on a PI plastic substrate via a series of wet chemical/electrochemical processes. The bottom Ni-P layer was deposited on a PI to replace conventional TCO as a conductive layer, and the top Ni3S2 layer was employed as the electrocatalyst for I3(-) reduction. On the basis of the extensive electrochemical measurments, the as-prepared Ni3S2/Ni-P coated PI flexible CE demonstrated a Pt-like electrocatalytic for I3(-) reduction. As a result, the DSC assembled with the Ni3S2/Ni-P coated PI flexible CE exhibited an impressive photovoltaic conversion efficiency of 6.28% accompanied by a fill factor of 0.63 under 1 sun illumination (100 mW cm(-2), AM 1.5), which is comparative to that of the DSC based on the Pt coated indium tin oxide/polyethylene naphthalate (ITO/PEN) CE.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Lin</LastName><ForeName>Jeng-Yu</ForeName><Initials>JY</Initials><Affiliation>Department of Chemical Engineering, Tatung University , No. 40, Sec. 3, ChungShan North Road, Taipei City 104, Taiwan.</Affiliation></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Wei-Yan</ForeName><Initials>WY</Initials></Author><Author ValidYN="Y"><LastName>Lin</LastName><ForeName>Yi-Ting</ForeName><Initials>YT</Initials></Author><Author ValidYN="Y"><LastName>Chou</LastName><ForeName>Shu-Wei</ForeName><Initials>SW</Initials></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType>Journal Article</PublicationType><PublicationType>Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2014</Year><Month>02</Month><Day>06</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Appl Mater Interfaces</MedlineTA><NlmUniqueID>101504991</NlmUniqueID><ISSNLinking>1944-8244</ISSNLinking></MedlineJournalInfo><CitationSubset>IM</CitationSubset></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="aheadofprint"><Year>2014</Year><Month>2</Month><Day>6</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2014</Year><Month>1</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2014</Year><Month>1</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2014</Year><Month>1</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="doi">10.1021/am405384c</ArticleId><ArticleId IdType="pubmed">24446929</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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